ORIGINALRESEARCHARTICLEDrugsRD2011;11(3):259-275

ª2011Websteretal.,publisherandlicenseeAdisDataInformationBV.Thisisanopenaccessarticlepublishedunder

thetermsoftheCreativeCommonsLicense‘‘Attribution-NonCommercial-NoDerivative3.0’’(

andreproduction,providedtheoriginalworkisproperlycitedandnotaltered.

ImpactofIntravenousNaltrexoneonIntravenousMorphine-InducedHigh,

DrugLiking,andEuphoricEffectsinExperienced,NondependentMaleOpioidUsers

LynnR.Webster,1FranklinK.Johnson,2JosephStauffer,2,3BeatriceSetnik2andSabrinaCiric4

1LifetreeClinicalResearch,SaltLakeCity,UT,USA

2AlpharmaPharmaceuticalsLLC,awhollyownedsubsidiaryofKingPharmaceuticalsInc.,Bridgewater,NJ,USA,acquiredby PfizerInc.inMarch2011

3JohnsHopkinsUniversitySchoolofMedicine, Baltimore,MD,USA

4Celerion,Montreal,QC,Canada

AbstractBackground:Opioidanalgesicscanbeabusedbycrushingfollowed by solu-bilizationandintravenousinjectiontoattainrapidabsorption.Morphinesulfateandnaltrexonehydrochlorideextendedreleasecapsules(EMBEDA®,

MS-sNT),indicatedformanagementofchronic,moderatetoseverepain,containpelletsofmorphinesulfatewithasequesterednaltrexonecore.Shouldproducttamperingbycrushingoccur,thesequesterednaltrexoneisintendedforreleasetoreducemorphine-inducedsubjectiveeffects.

Objective:Thisstudycomparedself-reportsofhigh,euphoria, and drug-likingeffectsofintravenousmorphinealoneversusintravenousmorphinecombinedwithnaltrexoneinaclinicalsimulationofintravenousabuseofcrushedMS-sNT.

Methods:Thissingle-center,randomized,double-blind,crossoverstudychar-acterizedsubjectiveeffectsofnaltrexoneadministeredintravenouslyatthesameratiotomorphinepresentinMS-sNT.Subjectsweremaleandhadusedprescriptionopioidsfiveormoretimeswithinthe previous12months toget‘high’butwerenotphysicallydependentonopioids.TheprimaryoutcomewastheresponsetotheDrugEffectsQuestionnaire(DEQ)question#5,‘‘Howhighareyounow?’’(100mmVisualAnalogScale[VAS]).Thesecondary

outcomewastheresponsetoaCole/AddictionResearchCenterInventory

(ARCI)Stimulation-Euphoriamodifiedscale.AdditionaloutcomesincludedresponsetoVASdrugliking,theremainingDEQquestions,andpupillometry.Results: Administration of intravenous naltrexone following intravenous

morphinediminishedmeanhigh(29.8vs85.2mm),Cole/ARCIStimulation-

Euphoria(13.7vs27.8mm),anddrug-liking(38.9vs81.4mm)scores(all

p0.0001)comparedwithintravenousmorphinealone.Noseriousadverse

eventsoccurredasaresultofthetestedratioofnaltrexonetomorphine.

Conclusions:Resultsinthisstudypopulationsuggestthatnaltrexoneaddedtomorphineinthe4%ratiowithinMS-sNTmitigatesthehigh,euphoria,and

druglikingofmorphinealone,potentiallyreducingtheattractivenessforproducttampering.Assessmentofthetrueclinicalsignificanceofthesefindingswill requirefurther study.

Introduction

Opioidanalgesicsareanimportantcomponentofcomprehensivemanagementplansforchronicpaininappropriatelyselectedandmonitoredpatients.Extended-releaseopioidformulationshaveenabledpatientstoattainaround-the-clockpainreliefwithlessfrequentdosingthanwithimmediate-releaseproducts;however,theyarevulnerabletotamperingbyabuserswishingtogainaccesstothelargersupplyofopioidwithineachdoseunit.[1,2]Forexample,someprescriptionopioidscanbeabusedbyinjectionof solubilizedcrushedproducttoachievetherapidabsorptionandhighopioidplasmalevelsassociatedwitha‘rush’or‘high.’[2]

Abuseofprescriptiondrugs,includingopioidanalgesics,hasincreasedsubstantiallysincethemid-1990s,[3-8]creatinganeedforproductsthatarealessinvitingtargetforabuse.[9-13]AmongUSDepartmentofHealthandHumanServices,FDA,CenterforDrugEvaluationandResearchrecommendationsisthecallfordrugmanufac-turersto‘‘modifyopioidpainkillerssothatthey

are moredifficult totamper withand/orcombine

them withagentsthatblock theeffect of theopioidifitisdissolvedandinjected.’’[14-16]Nal-trexonehydrochlorideisanorallyavailableopioidantagonistthatcompetitivelybindstom-opioid

receptors and reduces the euphoric effects of

m-opioidagonists,suchasmorphine.[17]Naltrexone,administeredgenerallyatdosesof50–100mg/dayfororaladministrationor380mg/monthforintra-

muscularadministration,isusedasanadjunctivetreatmentofalcoholismandforblockadeoftheeffectsof opioids.[18,19]Naltrexoneis also presentinamuchsmalleramountasasequesteredcomponentintheindividualpelletsinmorphinesulfateand

naltrexonehydrochlorideextendedreleasecap-sules(EMBEDA®,MS-sNT,formerlyALO-01).

MS-sNTisindicatedforthemanagementofchronic,moderatetoseverepain.[20]Theratioofmorphinesulfatetonaltrexonehydrochloridein

MS-sNTis100:4.[20] Thus,a30mgcapsuleof

MS-sNTcontains30mgofmorphinesulfateand

1.2mgofsequesterednaltrexone,anamountmuchlowerthantheaforementionedclinicaldosesofnaltrexone.

ThesequesteredcoreofnaltrexoneinMS-sNTisintendedforreleaseonlyuponproducttam-pering(crushing)toreducemorphine-inducedsubjectiveeffects.[20]PreviouspharmacokineticstudieshaddemonstratedthatwhenpelletsfromMS-sNTwerecrushedandtakenorally,boththemorphine and the naltrexonewerefully bioavail-ablewhencomparedwiththeequivalentamountofmorphineandnaltrexoneinsolution.[21,22]Resultsofanoralabuseliabilitystudyin32rec-reationaldrugusersindicatedthatMS-sNTcap-sules,takenorallyeitherwholeorwithliquidafterthepellets werecrushed,were significantlyless de-sirablethanmorphinesulfatesolution,aseval-

uatedusingseveralsubjectivemeasuresincludingCole/AddictionResearchCenterInventory(ARCI)

Stimulation-Euphoria,[23]drugliking,andsub-jectivemonetaryvalueofdrug.[21]Overall,87.5%

ofsubjectsintheoralstudyexperiencedsomedegreeofreduceddruglikingafterreceivingthecrushedMS-sNTcomparedwithmorphinesul-fatesolution.[20]

ThepurposeofthestudypresentedherewastoassesstheabuseliabilityofMS-sNTiftheproductwereabusedintravenously.Sincetheexcipientsinthecrushedoralformulationcouldcauseundueharmifinjectedintravenously,aclinicalsimula-tionwasperformed.Therelativehigh,euphoric,

anddrug-likingeffectsof30mgofintravenousmorphine alone versus 30mg of intravenous

morphinecombinedwith1.2mgofintravenousnaltrexone(100:4morphinesulfatetonaltrex-

onehydrochlorideratiocontainedinMS-sNTcapsules)wereassessedin recreationalopioidusers.ResultsmayfurtheraidincharacterizingtheabuseliabilityofMS-sNTandthepotentialtoreducedesirabilityforproducttampering.

Methods

Participants

Subjects were menaged 18–50 years whohadusedprescriptionopioidstoachievea‘high’atleastfivetimesinthelast12months,butwerenotphysicallyopioiddependent.Theywererecrea-tionalopioidabuserswhoonlyusedopioidsoral-lyorsnorted.Themostcommonlyabusedopioids

among thesubjectswereconsistentwith nationaldata[24]andincludedhydrocodone/acetaminophen,

oxycodoneimmediatereleaseandextendedre-lease,andmorphine. Subjectswhousedmultipledrugsexpressedapreferenceforopioids.Thesub-jectswererecruitedfromthedatabaseofLifetreeClinicalResearch(SaltLakeCity,UT,USA)andwerecompensatedfortheirtimeduringpartic-ipationinthestudy.

Subjectswereingenerallygoodhealthasas-sessedbymedicalhistoryandphysicalexamina-tion,laboratorytests,andECG,andhadnegativeurinedrugscreensforamphetamines,barbitu-rates,benzodiazepines,cocaine,andopioidsuponpresentationforadmissiontotheclinic.Subjectswithahistoryofsignificantneurologic,hepatic,renal,endocrine,cardiovascular,gastrointestinal,pulmonary,ormetabolicdiseasewereexcluded,aswerethosecurrentlyintreatmentforsubstanceabuseorwhohadcompletedasubstanceabuseprogramwithintheprevious90days.

Subjectscouldnothaveused,orhaveintendedtouse,anyprescriptionorover-the-counter(OTC)medicationsthatcouldinterferewiththeevaluationofmedicationduringthestudy.Prescriptionmedi-cationscouldnothavebeenusedwithin14daysofdosingandOTCmedicationscouldnothavebeenusedwithin48hoursofdosing.Subjectscouldnot

ingestalcohol,grapefruit,orgrapefruitjuicewithin48hoursofdosingorduringthestudy.

StudyDesign

Thissingle-center,randomized,double-blind,crossoverstudyincludedthefollowingthreephases:

(i)naloxonechallenge;(ii)drugdiscrimination;and

(iii)treatment.Itwasconducted inaccordance withthecurrentFDAregulations,International Con-ferenceonHarmonisationguidelines,GoodClin-icalPracticestandards, theDeclarationofHelsinki,andlocalethicalandlegalrequirements.[25,26]

NaloxoneChallengePhase

Analoxonechallengewasperformedonthedayofadmission(day0)toruleoutsubjectswhowerephysicallydependentonopioids.Subjectswereadministered0.1mgofintravenousnalox-one;iftherewerenosignsofopioidwithdrawalwithin30seconds,anadditional0.3mgofintra-venousnaloxonewasadministeredandsubjectswereobservedforwithdrawalsymptomsfor20min-utes.Subjectswereterminatedfromthestudyattheendofthenaloxonechallengephaseiftheyexhibitedsignsof opioidwithdrawal.

DrugDiscriminationPhase

Subjectswererandomizedtoreceiveonein-travenousinjectionofeither10mgofmorphineorplaceboon inpatientdays1and3 inadouble-blind,crossoverfashion,witha1-daywashoutonday2.Abilitytodistinguishmorphinefromplacebowasassessed bytheinvestigatorbasedon subjectresponsestoaDrugEffectsQuestionnaire(DEQ;

anine-itemquestionnairewitha100mmvisualanalogscale[VAS];0=none,100=extreme)[27]and the Cole/ARCI Stimulation-Euphoria modi-

fiedscale,descriptionfollowingintheStudyEndpointssection,atdesignatedtimepointsfol-lowingeachdose.[23,28]Attheconclusionofthedrugdiscriminationphase,theblindwasbroken.Theinvestigatordeterminedthesubjectswhowereabletodiscriminatebetweenmorphineandplaceboand,further,toreportamorepositiveoverall responsetomorphineversusplacebo, usingtheresponsetotheaforementionedstudyend-point measures,alongwithclinicaljudgment.

TreatmentPhase

Aftera1-daywashout(day4),subjectsenteredthetreatmentphase(days5–19)consisting ofthreetreatmentperiods.Duringeachtreatmentperiod,subjectsreceivedoneofthefollowingdosese-quences:(i)asingle30mgintravenousbolusofmorphineimmediatelyfollowedbyasingleintra-venousbolusofnaltrexoneplacebo;(ii)asingle30mgintravenousbolusofmorphineimmediatelyfollowedbyasingle1.2mgintravenousbolusofnaltrexone;or(iii)asingleintravenousbolusofmorphineplaceboimmediatelyfollowedbyasingleintravenousbolusofnaltrexoneplacebo.

Dosingswerespaced30secondsapart.There

wasa6-dayoutpatientwashoutbetweentreat-ments.Subjects wererequiredtohavea negativescreenfordrugsandalcoholonreadmissionforeachtreatmentperiod.

StudyTreatments

LifetreeClinicalResearchsuppliedstudytreat-mentsascommerciallyavailabledrugproductsforintravenous injection.Subjects,investigators,andthoseassessingtheoutcomeswereblindedtothestudydrug.Subjectswereassignedtotreat-mentinorderofenrollmentaccordingtoaran-domizationschedulegeneratedbythe statisticianandstoredinasecuredlocation.Thepharmacistwasresponsibleforcompletingamasterdrugaccountabilitylogdocumentinglotnumber,date,andtimeofdrugpreparation,anddateandtimeofdeliverytothestudycenter.Treatmentswereprovidedtostudycentersinprefilledsyringespackagedandlabeledwithprotocolnumber,date,andsubjectinitialsforthedrugdiscrimina-tionandtreatmentphases.AbbottLaboratories(NorthChicago,IL,USA)manufacturedthemorphinesulfate,KingPharmaceuticalsInc.(Bridgewater, NJ, USA) provided the naltrex-

onepowder,andBaxter(Deerfield,IL,USA)manufacturedthesodiumchloride0.9%sterile

diluent.

StudyEndpoints

Studyassessmentsincludedpharmacodynamic,pharmacokinetic,andsafetyendpoints.Ondos-

ingdaysduringthetreatmentphase,bloodsamplesforpharmacokineticmeasuresweredrawnatbaseline(beforedosing)andatsched-uledtimepoints(5minutesto24hourspost-dose).Pharmacodynamicoutcomeswereassessedimmediatelyfollowingeachpharmacokineticsampling.

The primary pharmacodynamic endpoint ofthisstudywasassessedbytheresponsetoDEQ

question#5,‘‘Howhighareyounow?’’[27] The

DEQcontainednineitemsorsubscales,eachpresentedasa100mmVAS.TheDEQquestionswereasfollows:(1)‘‘Doyoufeelanydrugef-fects?’’;(2)‘‘Doesthedrughavegoodeffects?’’;

(3)‘‘Doesthedrughavebadeffects?’’;(4)‘‘Doyoulikethedrug?’’;(5)‘‘Howhighareyounow?’’;(6)‘‘Doesthedrugmakeyoufeelsick?’’;

(7)‘‘Doyouhavenausea?’’;(8)‘‘Doesthedrugmakeyousleepy?’’;and(9)‘‘Doesthedrugmakeyoudizzy?’’Subjectswerefamiliarwithusingthe

DEQandtheCole/ARCIfromusing thesescales

duringthedrugdiscriminationphase.Thesecondaryendpointwasresponsetotheques-

tions on the Cole/ARCI Stimulation-Euphoria

subscalewhichconsistsof15statementsthatsub-jectsratedusinga4-pointscale(0–3,amod-

ificationofthe7-pointversion),where0=false,1=morefalsethantrue,2=moretruethanfalse,and 3=true. The total score is calculated by

addingtheindividualscores(maximumpos-sibletotalscore=45).[23,28]Sincethedrug-liking

VAShasbeenusedinotherstudiesasamea-

sureofdrugattractiveness,[21]datafromDEQquestion#4,‘‘Doyoulikethedrug?’’arereport-

edhere.DatafromtheremainingDEQsub-scales(#1–3and#6–9)andpupillometryarealso

summarized.

For pupillometry, lighting was controlledusingalightmetertoensurethatlightwasbetween

3.6luxand4.4lux.Pupildiameterwasmea-suredusingapupildensitometer,[29]withsmallervalues(pupillarymiosisorconstriction)indi-catingagreatermorphineeffect.End-tidalcar-bondioxidelevels,measuredbynoninvasivecapnography,wereassessednotasasafetyend-pointbutasanadditionalexploratorypharma-codynamicendpointandarenotincludedinthisreport.

AnalyticalMethods

Bloodsamples(approximately10mL)forphar-macokineticanalysiswerecollectedinVacutainer®

tubescontainingK2-ethylenediaminetetraaceticacidforassayofplasmamorphine,naltrexone,and6-b-naltrexol(themajornaltrexonemetabo-lite)concentrations.Immediatelyaftercollection,thetubesweregentlyinvertedtoensuremixingoftheanticoagulantwiththeblood;sampleswerepooled,splitintotwoaliquots,andkeptonice.Within45minutesofcollection,sampleswere

centrifugedat4°Cfor10minutesat3000revolu-

tionsperminute.Harvestedplasma(within30min-

utesofcentrifugation)wasstoredinanuprightpositionat-20–10°Cor colderin polypropylene

tubesuntilanalysis.Twocompletesetsoffrozensamples(aduplicatesetforbackup)wereprepared.Onecompletesetofsampleswascarefullypackedinapolystyreneshipperwithdryice,tightlysealed,andshippedviaovernightcourierto MDSPharmaServices(nowCelerion)[Lincoln,NE,USA]foranalysis.Theduplicatesetof sampleswas storedatLifetreeClinicalResearchuntilthesponsorprovideddirectionfordisposal.ConcentrationsoriginallycalculatedinconventionalunitswereconvertedtoSIunitstoallowdirectcomparisonofnumberofmoleculesofmorphineversusnaltrexoneand

6-b-naltrexol.Themolecularweightsusedforthecalculationsweremorphinemonomer285.34,naltrexone341.4,and6-b-naltrexol343.42(e.g.

toconvert50ng/mLmorphinetonmol/L,divide50ng/mL/molecularweightandmultiplyby1000,whichyields175nmol/L).Plasmaconcentrations

oftheanalytesweremeasuredusingvalidatedliquidchromatography-tandemmassspectrome-trywiththefollowinganalyticalranges:0.876–

175nmol/Lformorphine,0.0117–1.465nmol/Lfornaltrexone,and0.0116–4.66nmol/Lfor6-b-naltrexol. Samples with 0.0116nmol/L

6-b-naltrexolwerere-assayedwithamoresensi-tivemethod(range0.00146–0.0728nmol/L).

SafetyOutcomes

Safetywasevaluatedbyvitalsigns,pulseoxim-etry,physicalexaminations,ECGs,clinicallab-oratorytests,andadverseevents(AEs).Allsafety

analyseswerebasedonthedouble-blindsafetypopulationthatincludedallrandomizedsubjectswhoreceivedoneormoredosesofstudymed-ication(intravenousmorphine,intravenousnal-trexone,orintravenousplacebo)inthetreatmentphase.

StatisticalAnalysis

Samplesizewasdeterminedusingexperiencewithstudiesofsimilardesignthatevaluateddif-ferencesbetweenthetwoactivetreatments.Itwasexpectedthatapproximately76subjectswouldbescreened,with40participatinginthenaloxonechallenge,34continuingintothedrugdiscrim-inationphase,and24enteringthetreatmentphase.

Foreachsubjectinthepharmacodynamicpop-ulation(receivedoneormorestudytreatmentsinthedouble-blindtreatmentphaseandprovidedoneormoresubsequentpharmacodynamicassess-mentsduringthatphase),themaximum-effectscorewithinaperiod(Emax)andtimetomaximumeffect(TEmax)wereidentifiedforeachtreatmentperiod.Eachpharmacodynamicassessmentwassummarizedbytreatmentusingdescriptivesta-tisticsateachtimepoint.Inaddition,themeanforeachpharmacodynamicassessmentovertimewasplottedforeachtreatment.

WinNonlin® version 5.1 (Pharsight Corp.,

MountainView,CA,USA)wasusedtocalculateindividualsubjectpharmacodynamicoutcomes.All other analyses and tabulations were per-

formedusingSAS®version9.1.3(SASInstitute

Inc.,Cary,NC,USA)onaPCplatform.Eachpharmacodynamicassessmentwasanalyzedandp-valuesdeterminedusingalinearmixedmodel(PROCMIXED,SAS)withfixedeffectsforse-quence,period,andtreatmentarm,andarandomeffectforsubjectnestedinsequence.AdjustmentsformultiplecomparisonsweremadeusingtheBenjaminiandHochberg[30]methodinSASPROCMULTITEST.Leastsquares(LS)means

alongwith95%confidenceintervalswerepro-

vided foreachtreatmentarmand forall pairwisecomparisonsbetweentreatmentarms.TheEmaxwasusedforpharmacodynamicanalyses. TheEmax valueswereexpectedtobelog-normally

distributedandweretransformedpriortoanalysisbytakingthenaturallogarithm.Zerovalueswerereplacedwith0.0001asanarbitrarysmallvaluebecausealogtransformationisnotpossiblewithzerovalues.Descriptivestatisticsaswellasesti-

mates of geometric LS means and 95%con-

fidenceintervalswerecalculated.

The pharmacokinetic analyses were basedon all available post-dosing pharmacokinetic

data(n=28).Foreachsubject,thepharmaco-

kineticassessmentsweredeterminedusinganon-compartmentalapproachforallparametersinPhASTversion2.3-001software(1999;PhoenixAutomatedStatisticsandTabulation;manufac-turedbyPhoenixInternationalLifeSciences,locatedinMontreal,QC,Canada),exceptcon-centrationattime0[C0];C0wasestimatedwith

mentphase)included27subjects.Onesubjectwhohadcompletedthemorphineandtheplace-boarmswasdiscontinuedfornoncomplianceandhisdatawereexcludedfromtheevaluablepharmacodynamicpopulation.Asecondsubject,whowasincludedintheevaluablepharmacody-namicpopulation,wasdiscontinuedbeforecom-pletingplacebotreatmentduetoanAE(atoothinfectionunrelatedtostudydrug).

Inthesafetypopulation,theagerangewas18–36years(mean–standarddeviation:23.8–

4.5 years). Twenty-five subjects (89.3%) were

White,two wereAfricanAmerican,andonewasAsian.

Morphine

Morphine naltrexone

ADAPTIIRelease4(1997,BiomedicalSimula-

tionsResource,UniversityofSouthernCalifornia,LosAngeles,CA,USA).Summarystatisticsforplasmaconcentrationsofmorphine,naltrexone,and6-b-naltrexolwerecalculatedbytimeandtreatment.Fordataplotting,plasmaconcentra-tionvaluesthatwerebelowthelimitofquantifi-cation(BLQ)embeddedbetweentwomeasurableconcentrationsweresettomissing;however,BLQvaluesoccurringafterthelastmeasurableplasmaconcentrationweresettozero.Forthe

purposeofthecompartmentalpharmacokineticanalysis(C0calculations),allBLQvaluesoccur-ringafterthefirstmeasurableplasmaconcen-trationweresettomissing.

Results

Participants

Thestudywasconductedbetween20September2007and21November2007.Ofthe41subjectswhowerescreened,29wereenrolled.Onesubjectwhofailedthedrugdiscriminationphasewas

a

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0

b

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Placebo

0 1 2 3 4 5 6 7 8 9 10 11 12

discontinued.All28subjectsreceivingoneor

04812

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moredosesofstudydrugduringthedouble-blind

treatmentphasewereincludedinthepharmaco-dynamicandsafetypopulations.Theevaluablepharmacodynamicpopulation(completedthemorphineplusnaltrexonetreatmentandoneormoreothertreatmentsinthedouble-blindtreat-

Time post-dose (h)

Fig.1.Data(mean–standarddeviation)areshownfortheDrugEffectsQuestionnaire(DEQ)question#5,‘‘Howhighareyounow?’’afterintravenousadministrationofmorphine(n=28),morphineplusnaltrexone(n=27),andplacebo(n=27)asafunctionoftime(ordinate)

sincedrugadministrationinthepharmacodynamicpopulation.Datafor(a)12hoursand(b)24hourspost-dose.VAS=visualanalogscale.

TableI.Pharmacodynamicoutcomes

ParameterPlacebo(n=26)Morphine+naltrexone(n=27)Morphine(n=27)

DEQ#5:‘‘Howhighareyounow?’’(primaryoutcomemeasure)

Emax(mm)

meana–SD0.0–0.029.8–26.4b,c85.2–12.9c

range0–00–93.055.0–100.0

TEmax(h)

median0.00.10.1

range0–00–6.00.1–0.8

AUE2(h mm)

meana–SD0.0–0.022.4–28.2129.3–37.2

range0–00–115.532.3–191.3

AUE8(h mm)

meana–SD0.0–0.041.2–40.4315.0–160.5

range0–00–142.545.8–621.1

Cole/ARCIStimulation-Euphoria(secondaryoutcomemeasure)

Emax(mm)

meana–SD1.3–3.113.7–9.5b,c27.8–11.2c

range0–15.00–39.04.0–45.0

TEmax(h)

median0.00.10.3

range0–24.00–24.00.1–2.5

AUE2(mm unit)

meana–SD-0.2 –1.012.9–15.043.5–23.1

range-4.7to0.6-5.0to61.90.5–85.5

AUE8(mm unit)

meana–SD-0.9 –3.131.3–33.5118.3–73.6

range-14.7to0.1-21.5to113.40.5–250.1

DEQ#4:drugliking(additionaloutcomemeasure)

Emax(mm)

AUE2(mm.unit)

aArithmeticmean.

bp0.0001vsmorphine.c p0.0001vsplacebo.

ARCI=AddictionResearchCenterInventory;AUEx=areaundertheeffectcurvefromtime0toxhours;DEQ=DrugEffectsQuestionnaire;

Emax=maximumeffect;TEmax=timetomaximumeffect.

Morphine

Morphine naltrexone

aPlacebo

45

40

35

30

25

20

15

10

5

0

0 1 2 3 4 5 6 7 8 9 10 11 12

b

45

40

35

30

25

curve(AUE)wasgreaterwhenmorphinewasadministeredalonethanwhencoadministeredwithnaltrexone(seetableI).Themediandiffer-

enceinDEQ#5Emax scorebetweenmorphine

andmorphineplusnaltrexonewas62.0mm(range,7.0–93.0mm).Atmaximumeffect,only2of27

(7.4%)subjectsexperiencedlessthana10-point

difference.

TheresultsfortheCole/ARCIStimulation-

Euphoriasubscaleassessments(seetableIandfigure2)reinforcethefindingsoftheprimarypharmacodynamicassessmentof‘high’.MedianTEmaxformorphineplusnaltrexonewas0.1hourandformorphinewas0.3hours.ArithmeticmeanEmaxscoresweresignificantlygreaterformor-phinethanformorphineplusnaltrexoneorplacebo

Morphine

Morphine naltrexone

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15

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0

04812

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Placebo

Time post-dose (h)

Fig.2.Data(mean–standarddeviation)areshownfortheCole/AddictionResearchCenterInventory(ARCI)Stimulation-Euphoriasubscale scores after intravenous administration of morphine

(n=28),morphineplusnaltrexone(n=27),andplacebo(n=27)as

afunctionoftime(ordinate)sincedrugadministrationinthephar-macodynamicpopulation.Datafor(a)12hoursand(b)24hourspost-dose.

PharmacodynamicOutcomes

MeanDEQ#5(‘‘Howhighareyounow?’’)valuesovertimeareillustratedinfigure1.ThemedianTEmaxwas6minutes(0.1hour)forthemorphineandmorphineplus naltrexonetreat-ments,and0minutesforplacebo(seetableI).

Thearithmeticmean(–standarddeviation)score

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b

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0 1 2 3 4 5 6 7 8 9 10 11 12

fortheEmax wassignificantlygreaterformor- / 0 / 4 / 81216 / 20 / 24
phinethanmorphineplusnaltrexoneorplacebo / Time post-dose (h)

(85.2–12.9mmvs29.8–26.4mmvs0.0–0.0mm,

respectively;p0.0001).Thisdifferencewassta-

tisticallysignificantacrossallthreetreatmentgroupsaswellasbetweentreatmentgroupsinpairwisecomparisons.Meanareaundertheeffect

Fig.3.Data(mean–standarddeviation)areshownfortheDrugEffectsQuestionnaire(DEQ)question#4,‘‘Doyoulikethedrug?’’afterintravenousadministrationofmorphine(n=28),morphineplusnal-trexone(n=27), andplacebo(n=27)asa function oftime(ordinate)

sincedrugadministrationinthepharmacodynamicpopulation.Datafor(a)12hoursand(b)24hourspost-dose.VAS=visualanalogscale.

TableII.Exploratoryoutcome:pupillometry

AUE2(h mm)

meana–SD0.0–0.9-1.3–1.5-5.0–1.8

range-2.0to1.4-3.4to2.3-8.1to-1.4AUE8(h mm)

meana–SD0.3–4.8-8.5–6.8-18.8–8.0

range-10.6to9.1-19.1to6.4-32.7to-4.7a Arithmeticmean.

b p0.0001vsmorphine.c p0.0001vsplacebo.

AUEx=areaundertheeffectcurvefromtime0toxhours;Emin=minimumpupildiameter(maximumeffect);SD=standarddeviation;

TEmin=timetominimumpupildiameter(maximumeffect).

(27.8mmvs 13.7mm vs 1.3mm, respectively;p0.0001).MeanAUE wasgreaterwhen mor-

phinewasadministeredalonethanwhenad-ministeredwithnaltrexone(seetableI).Overall,

71%ofsubjectsreportedareductionineuphoria

withmorphineplusnaltrexonecomparedwithmorphinealone.[20]

ArithmeticmeanvaluesovertimeforDEQquestion#4, ‘‘Do you likethe drug?’’areshown

infigure3.MedianTEmaxformorphineplusnaltrexonewas0.1hourandformorphinewas

0.3hours.ArithmeticmeanscoreforEmaxfordruglikingwassignificantlygreaterformorphinethanmorphineplusnaltrexoneorplacebo(81.4mm

vs38.9mmvs0.0mm,respectively; p0.0001)

andmeanAUEwasgreaterwhenmorphinewasadministeredalonethanwhenadministeredwithnaltrexone (seetableI).

ForeachoftheremainingsevenDEQques-tions,theEmaxformorphinewasgreaterthanformorphineplusnaltrexoneandplacebo.Statisti-callysignificantgeometricmeandifferencesin

Emaxweredetectedacrossallthreetreatments(p0.0001).Forthe‘desirable’(positivesubjec-tiveeffects)DEQoutcomesof#1(drugeffects),

#2(feelinggoodeffects),and#4(likingthedrug),

themedianTEmaxwassimilarorslightlyshorterformorphinethanmorphineplusnaltrexone.MedianTEmaxvaluesforthe‘undesirable’(neg-

ativesubjectiveeffects)DEQoutcomesof#3(badeffects),#6(feelingsick),#7(havingnausea),#8(feelingsleepy),and#9 (feelingdizzy)wereearlier

for morphine plus naltrexonethanfor morphine.[21]

PupillometryAnalysis

Thepeakmorphinedrugeffectwasobservedwhenthepupildiameterwassmallest(indicativeofmorphine-inducedconstriction).MinimumpupildiameterisnotedasEmin,thebaselineforcom-parisonwhennotingincreaseinpupilsize.Fol-lowingintravenousadministrationofmorphinealone,themeanEmin(2.4mm)wassignificantlyreducedrelativetoplacebo(4.4mm)andmor-

phineplusnaltrexone(3.4mm)[p0.0001for

bothcomparisons].Mediantimetoreachthisminimumpupildiameter(TEmin)aftermorphinealonewasrapid(0.8hours)comparedwithpla-cebo(3.0hours)andmorphineplusnaltrexone(4.0hours).Themioticeffectwastemporallyde-layedrelativetomorphinealonewhenmorphinewasadministeredintravenouslywithnaltrexone.

MeanAUEfromtime0to8hoursformiosiswassmaller(-18.8h mmvs-8.5h mm)formorphine

alonerelativetomorphineplusnaltrexoneandplacebo(seetable IIandfigure4).

Pharmacokinetics

Plasmamorphineconcentration-timeprofilesandpharmacokineticparametersweresimilarforintravenousmorphinealonecomparedwithconcomitantintravenousnaltrexoneadministra-tion,includingextentofexposure(areaunderthe

Morphine

Morphine naltrexone

plasmadrugconcentration-timecurve)atthemeasuredtimepoints(seetableIIIandfigure5).Thissimilaritydemonstratedthatthecoadmin-istrationofnaltrexoneandmorphinehadnoap-parenteffectonthemorphinepharmacokineticswhen compared withmorphineadministered alone.Followingsingle intravenous bolus administrations,

morphine,naltrexone,and6-b-naltrexolreachedpeakconcentrationsimmediatelyafterdosingandthendecreasedinamulti-exponentialmanner(seefigure5).Pharmacokineticassessmentsofmor-phine,naltrexone,and6-b-naltrexolareshownintableIII.

a

7.0

6.5

6.0

5.5

5.0

4.5

4.0

3.5

3.0

2.5

0

b

7.0

6.5

6.0

5.5

5.0

4.5

4.0

3.5

3.0

2.5

Placebo

1 2 3 4 5 6 7 8 9 10 11 12

Pharmacokinetic-Pharmacodynamic

Relationship

Basedonadditionalexploratoryanalysis,figure6ashowsahysteresisplotofpercentagechangeineuphoriaabatementversusmeanplasma

naltrexoneconcentration using theCole/ARCI

Stimulation-Euphoriasubscaleovertime.Subjectswhodidnotexperienceeuphoria(18.5%,5of27)

werenotincludedintheanalysis.Theplasmanal-trexonerapidlyreacheditspeaklevel(21.4nmol/L)

by 5minutesandthendecreased.Thisisrelatedtoa median63%abatementofthemorphine-induced

euphoria.Thenaltrexone-inducedeuphoriaabate-mentcontinuedandreachedamaximumof80%by

30minutes.Figure6bshowstheincreaseinpupilsize (relative tothatwithmorphine)plotted againstplasmanaltrexoneconcentrationovertime.Themeannaltrexonepeakplasmalevelat5minutesisrelatedtoa2mmincreaseinpupilsizeshowingtheblockingofthemorphine-inducedpupilconstric-tion.Thiseffectwasmaintaineduntil45minutesandgraduallydecreasedinrelationtothelowerplasmanaltrexone levelsover time.

Safety

Inthisstudy,21of28(75%)subjectsexperi-encedatotalof69AEs.Nineteen(67.9%)sub-

jectsexperienced50oftheseAEswhentreated

0 2 4 6 8 10

12 14 16 18 20 22 24

withmorphinealone.Bycontrast,9of27(33.3%)

Time post-dose (h)

Fig.4.Pupillometrydata(mean–standarddeviation)overtime(phar-macodynamicpopulation).Datafor(a)12hoursand(b)24hourspost-dose.

subjectsexperienced17AEsduringtreatmentwithmorphineplusnaltrexoneandtwo(7.4%)

subjectstakingplaceboreportedtwoevents(seetableIV).ThemostfrequentlyreportedAEswere

TableIII.Summaryofpharmacokineticassessments

ParameterMorphinealone(n=28)Morphine+naltrexone(n=26)

C0(nmol/L)aAUC2(nmol.h/L)AUC8(nmol.h/L)

AUCt(nmol h/L)

a

AUC¥(nmol h/L)

t½(h)bVss(L)bCLt (L/h)b

aGeometricmean(CV%).

bArithmeticmean(SD).

AUCt=areaundertheplasmaconcentrationcurveattimet,wheretiseither12hoursor24hoursdependingonthetimeoflastmeasureableconcentration;AUC¥=areaundertheplasmadrugconcentration-timecurvefromtimezerotoinfinity;AUCx=areaundertheplasmadrugconcentration-timecurvefrom0toxhours;C0=anticipatedinitialplasmadrugconcentration;CLt=totalplasmaclearance;CV=coefficientofvariation;NA=notavailable;t½=terminalhalf-life;Vss=volumeofdistributionatsteadystate.

pruritus,nausea,andvomiting(seetableIV).Onesubject discontinuedbecause ofanAE(toothinfection).TherewerenodeathsorseriousAEs.Noclinicallysignificantabnormallaboratoryvalueswerereported.Onesubjectreportedamoderatelysevereepisodeofvasovagalsyncope,whichwasconsideredbytheinvestigatortobeunrelatedtostudydrugandresolvedsponta-neouslyonthedayofonset.Nostudydrug-relatedchangesinvitalsignsorphysicalfindingswerenoted.

Discussion

Thegoalofthisstudywastoassesstheintra-venousabuseliabilityofMS-sNTbysimulatingtheintravenousabuseoftheproductbyrecrea-tionalopioidabusers.Therelativeeffectsofin-travenous morphine alone or in combination

withintravenousnaltrexoneina100:4ratioon

high, euphoria,anddrug liking were assessed.

For the primary endpoint DEQ #5 (‘‘How

highareyounow?’’)maximumeffectachievedwithmorphinealonewasapproximately3-foldgreaterthanformorphineplusnaltrexone.Themaximum effectforplacebowas0.0mm.Onthe

Cole/ARCIStimulation-Euphoriasubscale,theeu-

phoriceffectofmorphinealonewasapprox-imatelytwicethatofmorphineplusnaltrexone.

Maximumeffectforboth treatments wassig-nificantlydifferentfromplacebo.Themaximumeffectfordruglikingofmorphinealonewasap-proximately2-foldgreaterthanformorphineplusnaltrexone.Resultsconsistentlydemonstrat-edgreatersubjectiveeffectswhenmorphinewastakenintravenouslyalonethanwhenitwasad-ministeredwiththenaltrexone.

The remaining pharmacodynamic analyses(DEQ#1–3and#6–9)demonstratedthat,inmost

instances,themeanmaximumvaluesformor-phinealoneweresignificantlygreaterthanthecorrespondingvaluesformorphineplusnaltrex-one andplacebo groups. ForeachDEQmeasure,morphineplusnaltrexoneprovidedsignificantlygreatereffectcomparedwithplacebo,butwithasufficientdosageofnaltrexonetosignificantlymitigatethemorphinesubjectiveeffects.Com-paredwithmorphinealone,thesubjectivelyap-pealingattributesofthedrug(suchasfeelingdrugeffects,feelinggoodeffects,andlikingthedrug)occurredmoreslowly,whiletheunappeal-ingattributesbecameevidentmorequicklyafterthemorphineplusnaltrexonecombination.Thissuggeststhatthepresenceofnaltrexonecontri-butedappreciablytotheabatementofmorphinehighandeuphoriawithoutdecreasingtheun-pleasanteffects(e.g.nausea,sleepiness)associatedwithmorphineuse.

Ananalysisperformedsubsequenttothisstudysuggestedthatdifferencesof8–10mminVASratingsof‘high’indicateclinicalsignificance.[31]Asshowninfigure1inthecurrentstudy,themeandifferenceinVASscoresforDEQquestion

#5,‘‘Howhighareyounow?’’observedbetween

morphineplusnaltrexoneand morphinealoneremained greater than 10mm from 5 minutes

Morphine and naltrexone

post-dosethrough8hourspost-dose.Atmax-imumeffect,only2of27(7.4%)subjectsexperi-

encedlessthana10-pointdifference.

Inthecontextofthisclinicalsimulation,thestudytreatmentswerewelltolerated.Itislikelythatadverseconsequenceswouldbemuchgreat-er incasesofparenteral abuseof MS-sNTduetothepresence of excipientssuch astalc.However,resultsof thisstudyshouldserve asan indicationthat,inadditiontothepotentialharmcausedbytamperingwithandinjectingMS-sNT,thede-

a

10 000

1000

100

10

1

0.1

Morphine

siredhighwouldnotbeattained.

Asmorphinecausesmiosis,[29,32,33]pupillo-metrymeasurementswereintroducedasanob-jectivemeasureofopioideffect.ThegeometricmeanEminwassignificantlysmallerafterintra-venousmorphinethanafterplacebooraftermorphineplusnaltrexone.Furthermore,theme-dianTEminwassignificantlyquickerwithmor-phinealonethanforplaceboormorphineplusnaltrexone.Inaddition,arelationshipwasobserv-edbetweenplasmanaltrexonelevelsandpupil

100

10

1

0.1

0.01

0.001

10

1

0.1

0.01

0.001

0

04812162024

b

04812162024

c

dilationovertimeinthehysteresisplot,showinganincreaseinpupilsize(relativetomorphinealone)of2mmformaximumnaltrexoneplasmalevelsafter5minutes.Thisfindingsuggeststhatthemorphine-induceddecreaseinpupildiameterwasinhibitedbynaltrexone.Thiseffect wassus-tainedfor45minutesandthengraduallyde-creasedastheplasmanaltrexonelevelsdecreased.Thepersistenceofasmallerpharmacodynamiceffect(continueddifferencebetweenmorphineandmorphineplusnaltrexone)overthere-mainderofthe12-hourperiodislikelycausedbyadoseeffectrelatedtoreceptorbinding.Therelativelysmallerdoseofnaltrexonecombinedwithhighhepaticclearancemayresultinreducedtemporaleffectfromthatofthemuchhigherdoseofmorphine.Thetimingofmorphine-inducedeffectsobservedinthisstudyisinagreementwiththatfromarecentlypublishedstudyin whichintra-

04812

162024

venousmorphinewasadministeredtointravenous-

Time post-dose (h)

Fig.5.Mean (mean–standarderror ofthe mean)plasmaconcen-tration-timeplotsforplasma(a)morphine,(b)naltrexone,and(c)6-X-

naltrexolafterintravenousadministrationofmorphine(n=28)ormorphineplusnaltrexone(n=26)asafunctionoftime(ordinate)

since drug administration in the evaluable pharmacodynamicpopulation.

experiencedrecreationalopioidusers.[34]

Apharmacokinetic-pharmacodynamicrelation-shipwasalsoobservedfortheplasmanaltrexonelevelsinrelationtothemorphine-inducedeupho-

riaasmeasuredbytheCole/ARCIStimulation-

Euphoriasubscale.Theplasmanaltrexoneversus

a

100

90

80

70

60

50

40

30

20

10

Time 0

0

2.50

2.25

2.00

1.75

1.50

1.25

1.00

0.75

0.50

0.25

03691215182124

b

0

Time 0

0.25

0369

1215182124

Plasma naltrexoneconcentration (nmol/L)

Fig.6.Dataareshownforthehysteresisplotof(a) percentagechangeineuphoriaabatementvs naltrexoneconcentrationovertime afteradministrationofintravenous(IV)morphinefollowedbyIVnaltrexone(n=22);and(b)increaseinpupilsizevsnaltrexoneconcentrationovertimeafteradministrationofIVmorphinefollowedbyIVnaltrexone(n=27).

euphoriaabatementandversuschangeinpupildiameterhysteresiscurvesvalidatesthenaltrexoneeffectonthesubjectiveresponses.

Althoughadministeredwithin30seconds,itispossiblethatthesequentialadministrationofmorphineandnaltrexoneallowedatemporary

TableIV.Mostfrequentlyreported(oneormore)adverseevents(AEs)[n(%)]

AE / Placebo(n=27) / Morphine+naltrexone(n=27) / Morphine(n=28)
Subjectsreporting‡1AE / 2(7.4) / 9(33.3) / 19(67.9)
Pruritus / 0(0.0) / 1(3.7) / 10(35.7)
Nausea / 1(3.7) / 3(11.1) / 9(32.1)
Vomiting / 0(0.0) / 1(3.7) / 7(25.0)
Headache / 0(0.0) / 4(14.8) / 2(7.1)
Dizziness / 0(0.0) / 2(7.4) / 3(10.7)
Nasaldiscomfort / 0(0.0) / 0(0.0) / 3(10.7)
Hiccups / 0(0.0) / 0(0.0) / 2(7.1)
Irritability / 0(0.0) / 0(0.0) / 2(7.1)
Dysuria / 0(0.0) / 0(0.0) / 3(10.7)

highasthedelayed effectofdisplacementofmorphinefromthem-opioidreceptorsfollowedbytheadministrationofnaltrexonetookplace.

IfpelletsfromMS-sNTcapsuleswerecrushed,dissolved,solubilized,and theninjected,both mor-phineandnaltrexonewouldbesimultaneouslyin-jected.Itwouldhavebeeninappropriatetoconductsuchastudywithcrushedpelletsduetotheconcernoverthepresenceofexcipientssuch astalc,butfu-turestudiesofthisnaturecouldincludesimulta-neousadministration.Additionalstudiesassessingbioavailabilityandsubjectiveresponsestoadmin-istrationoftamperedproductbyroutesotherthanintravenousororal(e.g.nasal)arealsowarranted.Thiscontrolledclinicalstudywasconductedinopioid-experienced, non-opioid-dependent menwho had not previously used the intravenousroutetoabusetheirdrugs.Selectionofthestudypopulationinhumandrug-abuseliabilitystudiesmayimpactoutcomesandpresentchallengesforwhichthereare fewestablished standards.[12,35,36]GuidancefromtheCenterforDrugEvaluationandResearchsuggeststhatsubjectsinastudyshouldhaveexperiencewithdrugswithpsycho-activepropertiessimilartothoseofthestudydrug, but do not specify route of administra-tion.[37]NationalAdvisoryCouncilon DrugAbuseguidelinesstatethatthe‘‘rationaleforexposuretonewdrugs,tohigherdoses,ortonewroutesof administration should be clear and compel-ling.’’[38]Forexample,onemayquestionwhethertheexperienceofintravenousadministrationofanopioidinsubjectswhohadnotpreviouslyused

thisroutetoabuseopioids mightencouragefutureopioidabuseby theintravenous route.Abuseliabilitystudiesinvolvingintravenousadminis-trationofthestudydrughavebeenperformedinnon-drug-abusingsubjects,intravenous-naivesubjects,andintravenous-experiencedabus-ers.[34,36,39,40]Asmallstudyreportedthatcocaineusepatternsdidnotchangeafterintravenous-naivesubjectsparticipatedinastudywithinves-tigationalintravenouscocaineadministration.[40]Kaufman,etal.[40]suggestedthatthisoutcomewasinfluencedbythefactthatthecontrolledclinicalsettinginwhichtheintravenousdrugwasadministeredduringthestudywasverydifferentfromthattypicallyassociatedwithintravenousdrugabuse.Overall,thefindingsfromthisandothersimilarly designed trials provideabasis forestablishingabuseliability.However,thesere-sultsarecenteredonasubsetofthepopulationofabusers(i.e.nondependentrecreationaldrugusers).Abuseliabilitymaydifferinothersubsetsofdruguserssuchasopioid-dependentindividualswho,upontampering,maybesusceptibletonaltrexone-precipitatedwithdrawal(e.g.patientswithchronicpainwhomisuseorabuseopioids,abusersaddictedto opioids,orto new initiatestoopioid abuse).AstudyisunderwaytodeterminetheeffectsofthequantityofnaltrexoneinMS-sNTonopioid-dependentindividuals.FuturestudiesareneededtoaddresstheoverallimpactthatMS-sNTandotherformulationsdesignedtoreduceattractive-nessforabusewillhaveonmisuse,abuse,anddiversioninthecommunity.

Conclusion

Opioidsareeffectiveandimportantinthetreatmentofchronic,moderatetoseverepaininappropriatelyselectedpatients;[41]however,inthecurrentclimateofincreasedillicituseofprescrip-tionopioidanalgesics,thereisaneedtoaddressthe goalofsuccessfully treatingpainwhilemini-mizingtherisksofabuse.[11]MS-sNTcapsulesprovideanalgesiawhentakenorallyasdirectedbutaredesignedtoreleasenaltrexoneiftheyaretamperedwithbycrushing.Resultsofthisintra-venousstudysuggestthattheratioofnaltrexonetomorphinewithinMS-sNTcapsulesissufficienttodecreasethesubjectiveeffectsofmorphineshouldMS-sNTpelletsbetamperedwithbycrushingandsolubilizedandtheninjectedintravenouslyinsubjectssimilartothestudypopulation.Thisfeaturemay reducethe consequentattractivenessofMS-sNTcapsulestotheseabusers.Assessmentofthetrueclinicalsignificanceofthesefindingswillrequirefurtherstudy.

Acknowledgments

LynnWebster,FranklinJohnson,JosephStauffer,andSabrinaCiricwereresponsible forthestudydesignandanal-ysis.Allauthorswereresponsible for analysisandinter-pretationofdata,conception,andwritingofthemanuscript,anddecisiontosubmitthemanuscriptforpublicationandapprovalofthefinalversion.

TheauthorsthankDonaldC.Manning,MD,PhD,andPaulF.CavanaughJr,PhD,formerlyofAlpharmaPharma-ceuticalsLLC(Bridgewater,NJ,USA),awhollyownedsub-sidiaryofKingPharmaceuticalsInc.,whichwasacquiredbyPfizerInc.inMarch2011,forcriticalreviewofthemanuscript;JodyM.Cleveland,MS,ofPfizerInc.(Cary,NC,USA)forstatisticalreviewandsupport;andBradBath,PhD,ofLife-treeClinicalResearch(SaltLakeCity,UT,USA)andTonyaMarmon,DrPH,ofSynteractInc.(Carlsbad,CA,USA)forscientificinput.Writingandeditorialsupportforthismanu-scriptwasprovidedbyCarolBerry,MSc,andJessicaKrauklis,BS,ofQuintilesMedicalCommunications(Parsippany,NJ,USA)incloseconsultationwiththeauthorsandfundedbyPfizerInc.

LynnR.WebsterhasreceivedfundingfromKingPhar-maceuticalsInc.,which wasacquired byPfizer Inc.inMarch2011,forclinicalresearch,consulting,andparticipationinadvisoryboards.Hehasalsoreceivedfundingforclinical

researchand/orconsulting,honoraria,andparticipation in

advisoryboardsfromAdolorCorp.;Alkermes,Inc; Allergen,Inc;AmericanBoardofPainMedicine;Astellas;AstraZeneca;BayerHealthcare;BioDeliverySystemsInternational;BostonScientific;CephalonInc;CollegiumPharmaceuticals;Covidien;

CovidienMallinkrodt;Eisai;ElanPharmaceuticals;GileadSciences;GlaxoSmithKline;JanssenPharmaceuticalK.K.;MeaganMedical;Medtronic;Nektar Therapeutics;NeurogesX,Inc;NevroCorporation;Pharmacofore,Inc.;PurduePharma;ShionogiUSA.Inc.;StRenatus;SuCampoPharmaAmericas,USA;TEVAPharmaceuticals (Sub-1); Theravance;Theravance,Inc;Vertex;andXanodynePharmaceuticals.FranklinK.JohnsonisaformeremployeeofAlpharmaPharmaceuticalsLLC,awhollyownedsubsidiaryofKingPharmaceuticalsInc.,whichwasacquiredbyPfizerInc.inMarch2011,and

ownedstockinAlpharmaPharmaceuticalsLLC.Heisalsoa coinventor of EMBEDA® technology. Joseph Stauffer

isaformeremployeeofAlpharmaPharmaceuticalsLLC,awhollyownedsubsidiaryofKingPharmaceuticalsInc.,whichwasacquiredbyPfizerInc.inMarch2011,andownsstockoptions and patents for Alpharma Pharmaceu-ticalsLLC.BeatriceSetnikisanemployeeofPfizerInc.andownscompanystocksinKingPharmaceuticalsInc.SabrinaCiricisanemployeeofCelerion(formerlyMDSPharmaServices),whichperformedtheanalyticalservicesforthisstudy.

ThisstudywassponsoredbyAlpharmaPharmaceuticalsLLC,awhollyownedsubsidiaryofKingPharmaceuticalsInc.,whichwasacquiredbyPfizerInc.inMarch2011.

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Correspondence:LynnR.Webster,MD,MedicalDirector,LifetreeClinicalResearch,andSeniorConsultanttoOmegaPainClinic,3838South700East,Suite200,SaltLakeCity,UT84106,USA.

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