Support information (SI)

Bulk atmospheric deposition of persistent toxic substances (PTS) along environmental gradients in Brazil

Rodrigo Ornellas Meire

João Paulo Machado Torres

Biophysics Institute, Rio de Janeiro Federal University, CCS, 21941-902 Rio de Janeiro, Brazil;

I. 1 Figure

Figure S1: PU deposition systems

II. 3 Tables

Table S1 - Description of sampling sites and exposure periods

Table S2 – Range and median concentrations for OCs deposition rates (pg.m-2.day-1) along different environment gradients.

Table S3 Range and median concentrations for PCB deposition rates (pg.m-2.day-1) along different environment gradients.

Figure S1 – PU deposition system

Table S2 – Range and median concentrations for OCs deposition rates (pg.m-2.day-1) along different environment gradients.
Urban / Suburban / Rural / Background
HCB / 213 / 60 / 18 / 49
α-HCH / 257 / 57 / 38 / 63
γ-HCH / 75 / 33 / 36 / 165
β-HCH / 26 / 137 / 128 / 129
Heptachlor / 287 / <43 / <43 / <43
Heptx / 561 / <37 / <37 / <37
Aldrin / <39 / <39 / <39 / 57
Endrin / <30 / <30 / <30 / <30
Dieldrin / 788 / <34 / 55 / <34
G clord / <5 / 50 / 36 / 35
A clord / <4 / <4 / <4 / <4
Endo-I / 112 / 33 / 28 / 16
Endo-II / <10 / 161 / 546 / <10
Metoxichlor / 382 / <4 / <4 / <4
pp-DDD / 613 / 25 / 80 / 15
op-DDD / <3 / 190 / 88 / <3
pp-DDE / 1017 / BDL / 44 / <2
op-DDE / <45 / <45 / <45 / <45
pp-DDT / 3408 / 620 / 229 / <50
op-DDT / <15 / <15 / <15 / <15
ΣHCH / 483 / 523 / 202 / 360
ΣEndo / 116 / 195 / 573 / 31
ΣDDT / 6030 / 835 / 454 / 54
*Urban sites – Rio de Janeiro, Santa Catarina and Acre states; Suburban sites – Rio de Janeiro and Santa Catarina States; Rural sites – Santa Catarina States; Background sites – Rio de Janeiro and Santa Catarina States. ( < ) – Below detection limits.
Table S3 Range and median concentrations for PCB deposition rates (pg.m-2.day-1) along different environment gradients.
Urban / Suburban / Rural / Background
PCB-8 / 105 / <30 / <30 / <30
PCB-18 / 182 / 377 / 208 / 133
PCB-28 / <6 / <6 / <6 / <6
PCB-52 / 646 / 313 / 251 / 600
PCB-44 / 845 / 394 / 301 / 737
PCB-66 / 1475 / 800 / 626 / 1362
PCB-77 / 1870 / 721 / 594 / 1020
PCB-81 / 926 / 380 / 306 / 544
PCB-101 / 1273 / 636 / 535 / 983
PCB-105 / 547 / 192 / 162 / 230
PCB-114 / 298 / 167 / 107 / 200
PCB-118 / 891 / 290 / 240 / 341
PCB-123 / <30 / 400 / 367 / 536
PCB-126 / 199 / 62 / 61 / 82
PCB-128 / 64 / 60 / 48 / 67
PCB-138 / 1186 / 344 / 326 / 438
PCB-153 / 989 / 340 / 321 / 1060
PCB-156 / 189 / 60 / 63 / 70
PCB-157 / 43 / 150 / 63 / 8
PCB-167 / 256 / 60 / 47 / 67
PCB-169 / <13 / <13 / 24 / <13
PCB-170 / 255 / 67 / 70 / 74
PCB-180 / 509 / 132 / 138 / 162
PCB-189 / 17 / 6 / 6 / 8
PCB-195 / 31 / 7 / 11 / <2
PCB-206 / <7 / <7 / <7 / <7
PCB-209 / 6 / <2 / <2 / <2
ΣPCB / 13090 / 6040 / 4960 / 8230
ΣPCBind / 4600 / 2290 / 1580 / 2616
*Urban sites – Rio de Janeiro, Santa Catarina and Acre states; Suburban sites – Rio de Janeiro and Santa Catarina States; Rural sites – Santa Catarina States; Remote sites – Rio de Janeiro and Santa Catarina States. ( < ) – Below detection limits.