Methodology for Deriving Standards
for Contaminants in Soil
to Protect Human Health
This report may be cited as:
Ministry for the Environment. 2011. Methodology for Deriving Standards for Contaminants in Soil to Protect Human Health. Wellington: Ministry for the Environment.
Published in June 2011 by the
Ministry for the Environment
Manatū Mō Te Taiao
PO Box 10362, Wellington 6143, New Zealand
ISBN:978-0-478-37237-3
Publication number: ME 1055
Other publications in this series include:
Toxicological Intake Values for Priority Contaminants in Soil
© Crown copyright New Zealand 2011
This document is available on the Ministry for the Environment’s website:
Acknowledgements
This report was prepared for the Ministry for the Environment by Graeme Proffitt (Pattle Delamore Partners Limited).The sections of the report relating to plant bioconcentration factors for each contaminant, and produce consumption (Appendix 3), were derived from reports prepared by Jo-Anne Cavanagh (Landcare Research).
The advice and assistance of the Ministry’s Technical Advisory Group for this report is acknowledged.The members were:
Gerald Rys – Ministry of Agriculture and Forestry
Jim Waters – Environmental Risk Management Authority New Zealand
John Reeves – New Zealand Food Safety Authority
Marcus Hermann – Auckland City Council
Martin Robertson – Shell Oil
Mervyn Chetty – Auckland City Council
Murray Parrish – Carter Holt Harvey
Natalia Foronda – Ministry of Health
Nick Kim – Environment Waikato
Contents
Acknowledgements
Executive Summary
1Introduction
1.1Background
1.2Purpose
1.3Document organisation
2General Approach to Deriving Soil Guideline Values
2.1Concepts in risk assessment
2.2Generic equations
2.3Generic exposure scenarios
3Exposure Scenarios
3.1Scenarios adopted
3.2Scenarios not adopted
4Derivation Equations
4.1General
4.2Background exposure
4.3SGV(health) derivation equations for each pathway
4.4Soil ingestion
4.5Dermal absorption
4.6Produce ingestion
4.7Inhalation
5Exposure Parameters
5.1General
5.2Degree of conservatism
5.3General exposure parameters
5.4Pathway-specific parameters
5.5Contaminant-specific factors
5.6Summary of exposure factors
6Soil Contaminant Standards for Selected Priority Contaminants
6.1Arsenic
6.2Boron
6.3Cadmium
6.4Chromium
6.5Copper
6.6Inorganic lead
6.7Inorganic mercury
6.8Benzo(a)pyrene (BaP)
6.9DDT
6.10Dieldrin
6.11Dioxin and dioxin-like PCBs
6.12Pentachlorophenol
7Summary of Soil Contaminant Standards and Guideline Values
8Limitations of Soil Contaminant Standards
9Site-specific Risk Assessment
9.1Purpose
9.2Introduction
9.3When a site-specific assessment should not be carried out
9.4When a site-specific assessment must be carried out
9.5When a site-specific assessment may be carried out
9.6What factors may be changed?
9.7The site-specific assessment process
Appendices
Appendix 1:Detailed Calculations
Appendix 2:Detailed SGV(health) Calculations for Cadmium
Appendix 3:Determination of the Amount of Produce Consumed and its Dry Weight
Appendix 4:Dioxin SGV(health) Calculations with Egg Consumption
Appendix 5:International Comparison of Soil Guideline Value Derivation
Appendix 6:Natural Background Topsoil Datasets for Arsenic and Cadmium
Abbreviations and Glossary
References
Tables
Table ES1:Summary of soil contaminant standards – SCSs(health) – for inorganic substances (mg/kg)
Table ES2:Summary of soil contaminant standards – SCSs(health) – for organic compounds (mg/kg1)
Table 1:Scenarios for generic numeric values in various jurisdictions
Table 2:Parks / recreation scenarios – recommended approaches
Table 3:Age ranges and body weights of receptors considered in national and international derivation protocols
Table 4:Comparison of daily soil intake for recreational scenarios
Table 5:Soil ingestion rates used in national and international protocols
Table 6:Summary of child soil ingestion rate recommendations as reviewed
Table 7:Default soil ingestion rates for child and adult (mg/day)
Table 8:Produce consumption rates (g FW/day) used in international protocols
Table 9:Default produce consumption rates: weights in grams with percentage of total vegetables given in parenthesis
Table 10:Area of exposed skin and body parts considered to be exposed for different receptors, used in national and international protocols
Table 11:Body parts exposed for a child and associated skin areas (cm2)
Table12:Estimated soil adherence factors (mg/cm2)
Table13:Soil adherence values (mg/cm2)
Table 14:Summary of daily inhalation rates in existing New Zealand and international guidelines (m3/day)
Table 15:Inhalation rates recommended in Exposure Factors Handbook
Table 16:General and scenario-specific exposure parameters
Table 17:BCF for arsenic from different sources
Table 18:Contaminant-specific parameters for the derivation of the arsenic soil contaminant standard
Table 19:Arsenic soil contaminant standard (mg/kg)
Table 20:Contaminant-specific parameters for the derivation of the boron soil contaminant standard
Table 21:Boron soil contaminant standard (mg/kg)
Table 22:Coefficients determined for equations 23 and 24, and the percentage of the variability in the data
Table 23:Coefficients determined for equation 24, and the percentage of the variability in the data explained using an extended data set
Table 24:Contaminant-specific parameters for the derivation of the cadmium soil contaminant standard
Table 25:Cadmium soil contaminant standard (mg/kg)
Table 26:Summary of BCFs for chromium from different sources
Table 27:Contaminant-specific parameters for the derivation of the chromium soil contaminant standard
Table 28:Chromium III soil contaminant standard (mg/kg)
Table 29:Chromium VI soil contaminant standard (mg/kg)
Table 30:Contaminant-specific parameters for the derivation of the copper soil contaminant standard
Table 31:Copper soil contaminant standard (mg/kg)
Table 32:Recommended BCF (dry weight) and BCF (dry weight) for lead from different sources
Table 33:Contaminant-specific parameters for the derivation of the lead soil contaminant standard
Table 34:Lead soil contaminant standard (mg/kg)
Table 35:BCF for mercury from different sources
Table 36:Contaminant-specific parameters for the derivation of the inorganic mercury soil contaminant standard
Table 37:Inorganic mercury soil contaminant standard (mg/kg)
Table 38:Contaminant-specific parameters for the derivation of the BaP soil contaminant standard
Table 39:BaP soil contaminant standard (mg/kg)
Table 40:PEFs for use in assessing potential carcinogenicity of PAH mixtures
Table 41:BCF (geometric mean) for p,p’-DDT and p,p’-DDE in root and leafy vegetables determined from the literature
Table 42:Contaminant-specific parameters for the derivation of the DDT soil contaminant standard
Table 43: DDT soil contaminant standard (mg/kg)
Table 44:Contaminant-specific parameters for the derivation of the dieldrin soil contaminant standard
Table 45: Dieldrin soil contaminant standard (mg/kg)
Table 46:WHO (2005) TEFs for dioxins and dioxin-like PCBs
Table 47:BCF for dioxins and dioxin-like PCBs from Inui et al (2008), Hulster et al (1994) and recommended BCFs
Table 48:Contaminant-specific parameters for derivation of the dioxin and dioxin-like soil contaminant standards
Table 49:Dioxin and dioxin-like PCB soil contaminant standards (µg TEQ/kg)
Table 50:Egg lipid / soil ratios for PCDD/PCDFs and dioxin-like PCBs
Table 51:Dioxin and dioxin-like PCB soil guideline values for egg consumption pathway (µg TEQ/kg)
Table 52:Contaminant-specific parameters for the derivation of the PCP soil contaminant standard
Table 53:PCP soil contaminant standard (mg/kg)
Table 54:Summary of soil contaminant standards (shaded) and guideline values for inorganic substances (unshaded) (mg/kg)
Table 55:Summary of soil contaminant standards (shaded) and guideline values for organic compounds (unshaded)
Table 56:Modifiable exposure factors, typical situations and examples
Table A1.1:General and scenario-specific exposure parameters
Table A3.1:Amount of fruit and vegetables consumed (grams per day) by different age-gender groups based on simulated diets for the New Zealand 2003/04 Total Diet Surveys
Table A3.2:Vegetables considered in simulated diets, and their grouping
Table A3.3:Fresh to dry conversion factors for vegetables
Table A3.4:Amounts of different vegetable groups consumed by an average adult and average child, with percentage of total vegetables given in parenthesis
Table A5.1:Summary of the name / terminology used, purpose, and basis for derivation of soil guideline values in different countries
Table A5.2:Summary of USEPA exposure pathways of concern for residential and commercial / industrial land uses, and construction for deriving SSLs
Table A5.3:Exposure scenarios in existing New Zealand industry-based guidelines
Table A6.1:Regional council supplied data
Table A6.2:National statistics of the natural arsenic background concentration in topsoil
Table A6.3:Statistics of the natural arsenic background concentration in topsoil by region
Table A6.4:Summary statistics of the national natural background cadmium topsoil dataset
Table A6.5:Arsenic background sites in native bush
Table A6.6:Cadmium background sites
Figures
Figure 1:Pathway for subsurface vapour intrusion into indoor air
Figure 2:Life expectancy at birth, 1876–2002
Figure 3:Variation in plant bioconcentration factors (BCF, dry weight) for leafy vegetables with soil concentration and pH
Figure 4:Variation in plant bioconcentration factors (BCF, dry weight) for root and tuber vegetables with soil concentration and pH
Figure 5:Dependence of cadmium soil contaminant standard on pH
Figure 6:Site-specific assessment steps
Figure A2.1:Dependence of cadmium soil guideline value on pH
Figure A5.1:Derivation of screening values based on different risk levels and applications
Figure A5.2:Overview of steps for derivation of a soil quality guideline in Canada
Figure A5.3:Assumed soil allocation factor from the residual tolerable daily intake
Figure A5.4:Schematic lay-out of the CSOIL exposure model
Executive Summary
This technical report sets out a risk-based methodology for deriving soil contaminant concentrations protective of human health. Together with the Toxicological Intake Values for Priority Contaminants in Soil(MfE, 2011),this document serves as a technical referencein support of the National Environmental Standard for Assessing and Managing Contaminants in Soilto Protect Human Healthand should be read in conjunction with it (see
This report addresses a question that is fundamental to the science of contaminated land management: What contaminant concentration in soil can people be exposed to and yet not be subject to an appreciable risk of harm?The answer to this question varies internationally because each jurisdiction frames its response to fit within unique risk policy and legislative frameworks. So, although the technical approach to risk assessment of contaminated land is shared broadly by most countries, there are significant differences in detail such that a standard adopted by one country may not suit another.
As an alternative to adopting standards from another country, the Ministry for the Environment has examined the science of risk assessment and compiled a derivation methodology for health-based standards to apply to soil contaminants in New Zealand under the Resource Management Act 1991. This initiative comes at a time when it is appropriate also to review the soil guideline values contained within the Ministry’s existing suite of contaminated land guidelines. The ‘soil contaminantstandards’contained in this technical report are intended to supersede the ‘soil acceptance criteria’ used in previous New Zealand guidelines; the new methodology also resolves technical differences between them.The Ministry intends to apply the same approach when reviewing the petroleum hydrocarbon contaminants.
The term ‘soil contaminant standards’ to protect human health, or SCSs(health),specifically refers to soil contaminant concentrations that are mandatory, under the National Environmental Standard for Assessing and Managing Contaminants in Soilto Protect Human Health. SCSs(health)may be applied as Tier 1 or screening criteria; as conservative clean-up targets, to inform on-site management actions; or to trigger further investigation within a Tier 2 assessment. When talking about generic numerical values in guidelines or foreign jurisdictions, or for soil contaminant concentrations that are derived on a site-specific basis according to this methodology, the term soil guideline values (SGVs) is used.
If SCSs(health)or SGVs(health) are exceeded, it may result in health effects that are more than minor for some people, and as such are unacceptable.Conversely, if actual soil concentrations are less than or equal to the SCSs(health) or SGVs(health)then this is judged to be acceptable, because any adverse effects on human health for most people are likely to be no more than minor.
The methodology in this document is government policy and has two applications. First it demonstrates how the standards for contaminants in soil were derived for use within the NES regulation as ‘soil contaminant standards’, SCSs(health). Secondly, it sets out the basis for deriving soil contaminant concentrations protective of human health for exposure scenarios that lie outside of the generic exposure scenarios under the NES. The purpose of this second application of the methodology is to guide the site-specific derivation of soil guideline values, SSGVs(health), when there is good reason to use a site-specific risk assessment.
It is important to note that the methodology and the derived standards are intended to be protective of human health only, and do not apply to other environmental receptors.When it is relevant to protect other valued elements of the environment, separate consideration of appropriate values to achieve this is required.
This report presents:
- a national risk-based methodology for deriving soil contaminant concentrations protective of human health
- a suite of numerical criteria for priority contaminants that are legally binding as gazetted under the National Environmental Standard for Assessing and Managing Contaminants in Soilto Protect Human Health
- background information on the risk assessment methodologies and exposure parameters.
SCSs(health)are derived for the following priority contaminants:arsenic, boron, cadmium, chromium, copper, inorganic lead, inorganic mercury (but not elemental mercury), benzo(a)pyrene (representing the carcinogenic polycyclic aromatic hydrocarbons), DDT (as the sum of DDT, DDD and DDE), dieldrin, dioxin (as 2,3,7,8-tetrachlorodibenzo-p-dioxin (TCDD) and dioxin-like polychlorinated biphenyls (PCBs)), and pentachlorophenol (PCP).
The SCS(health)calculations draw on toxicological intake values and background exposures set out in the companion document,Toxicological Intake Values for Priority Contaminants in Soil(MfE, 2011).Numerical values are calculated for five generic land-use scenarios, and utilise standardised receptors and exposure parameters.
A summary of the SCSs(health) derived is presented in Tables ES1 and ES2.Contaminated-land practitioners are referred to the more detailed version of these tables set out in section 7 of this report, in which additional residential sub-scenarios have also been derived.
Table ES1:Summary of soil contaminantstandards– SCSs(health)– for inorganic substances (mg/kg)
Arsenic / Boron / Cadmium (pH 5)1 / Chromium / Copper / Inorganiclead / Inorganic mercuryIII2 / VI
Rural residential / lifestyle block 25% produce / 17 / NL / 0.8 / NL / 290 / NL / 160 / 200
Residential 10% produce / 20 / NL / 3 / NL / 460 / NL / 210 / 310
High-density residential / 45 / NL / 230 / NL / 1,500 / NL / 500 / 1,000
Recreation / 80 / NL / 400 / NL / 2,700 / NL / 880 / 1,800
Commercial / industrial outdoor worker / 70 / NL / 1,300 / NL / 6,300 / NL / 3,300 / 4,200
1Default value is for pH 5. Values increase with increasing pH (see Appendix 2).
2The SCSs(health) for boron, chromium III and copper represent levels well in excess of concentrations that would affect the health of plants.
NL = No limit. This is where the derived values exceed 10,000 mg/kg.
Table ES2:Summary of soil contaminantstandards– SCSs(health)– for organic compounds (mg/kg1)
Scenario / BaP / DDT / Dieldrin / PCP / Dioxin (µg/kg TEQ)TCDD / Dioxin-like PCBs
Rural residential / lifestyle block 25% produce / 6 / 45 / 1.1 / 55 / 0.12 / 0.09
Residential 10% produce / 10 / 70 / 2.6 / 55 / 0.15 / 0.12
High-density residential / 24 / 240 / 45 / 110 / 0.35 / 0.33
Recreation / 40 / 400 / 70 / 150 / 0.6 / 0.52
Commercial / industrial outdoor worker / 35 / 1,000 / 160 / 360 / 1.4 / 1.2
1All values in mg/kg dry weight except dioxins which are in µg/kg.
Methodology for Deriving Standards for Contaminants in Soil to Protect Human Health1
1Introduction
1.1Background
The Ministry for the Environment (MfE) has determined the need for a better policy framework for managing contaminated land in New Zealand.After extensive public consultation, the Ministry published a position paper in September 2007 (MfE, 2007).The paper identified, among other things, an inconsistent and variable use by contaminated-land practitioners of numerical contaminatedland guidelines used to assess the risk that contaminated soil might pose to human health.The Ministry then determined that, as a matter of priority, it would develop:
- a national risk-based methodology for deriving soil contaminant concentrations protective of human health
- a suite of numerical criteria for priority contaminants as examples of the national methodology
- site management options and actions that follow from applying the above criteria; ie, the numerical criteria may:
serve as Tier 1 or screening criteria to assess whether there is a potential risk to human health
when the numerical criteria are exceeded, serve as conservative clean-up targets for many situations, ie, where further investigation or site-specific risk assessment is not warranted or economic
inform on-site management actions to reduce the potential for adverse effects
trigger further investigation to better assess the risk and/or determine site-specific criteria as a Tier 2 assessment.
The Ministry intends that the derivation methodology be incorporated by reference into the National Environmental Standard for Assessing and Managing Contaminants in Soilto Protect Human Health (NES), as was proposed in the Discussion Document (Proposed National Environmental Standard for Assessing and Managing Contaminants in Soil, MfE, 2010a).While the technical detail behind the newly derived soil contaminantstandards is presented within this separate methodology document, the soil contaminantstandards will be applied in accordance with the NES and within the context of the derivation methodology.
This technical report introduces and sets out the risk-based methodology the Ministry has adopted as government policy for deriving SCSs(health): soil contaminantstandardsto protect human health.SCSs(health) are derived for a limited group of priority contaminants that are of primary concern in New Zealand. These are specifically: arsenic, boron, cadmium, chromium, copper, inorganic lead, inorganic mercury, benzo(a)pyrene, DDT, dieldrin, pentachlorophenol, and dioxin (as 2,3,7,8-tetrachlorodibenzo-p-dioxin, and dioxin-like polychlorinated biphenyls). These calculations draw on toxicological values and background exposures set out in a companion document Toxicological Intake Values for Priority Contaminants in Soil (MfE, 2011).
The numerical values are restricted to consideration of human-health risks and are based on conservative standard land-use scenarios, using standardised receptors and exposure parameters.